Maybe I can unwrap again and place directly over old unwrapped eye on Image ?
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Yes, you can. Unwrap them, resize the pieces and put them on the same area or a free area of the map where there is room enough for them, and paint them again (you will have to deal with all steps that affect the eyes, I mean normals, cavity, roughness, emission… everything you had applied to them). Just be extremely careful when selecting maps and selecting that the every new bake does NOT replace the whole corresponding map.
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Excellent !!! Thanks … 
Ill get on with it then … 
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